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In-MOF-derived In2S3/Bi2S3 heterojunction for enhanced photocatalytic hydrogen production

《能源前沿（英文）》 2023年 第17卷 第5期   页码 654-663 doi: 10.1007/s11708-023-0885-5

摘要： Transition metal sulfides are commonly studied as photocatalysts for water splitting in solar-to-fuel conversion. However, the effectiveness of these photocatalysts is limited by the recombination and restricted light absorption capacity of carriers. In this paper, a broad spectrum responsive In2S3/Bi2S3 heterojunction is constructed by in-situ integrating Bi2S3 with the In2S3, derived from an In-MOF precursor, via the high-temperature sulfidation and solvothermal methods. Benefiting from the synergistic effect of wide-spectrum response, effective charge separation and transfer, and strong heterogeneous interfacial contacts, the In2S3/Bi2S3 heterojunction demonstrates a rate of 0.71 mmol/(g∙h), which is 2.2 and 1.7 times as much as those of In2S3 (0.32 mmol/(g∙h) and Bi2S3 (0.41 mmol/(g∙h)), respectively. This paper provides a novel idea for rationally designing innovative heterojunction photocatalysts of transition metal sulfides for photocatalytic hydrogen production.

关键词： photocatalytic hydrogen production     wide-spectrum response     metal sulfides     MOFs derivative     heterogeneous interfacial contact    

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Interfacial induction and regulation for microscale crystallization process: a critical review

《化学科学与工程前沿（英文）》 2022年 第16卷 第6期   页码 838-853 doi: 10.1007/s11705-021-2129-8

摘要： Microscale crystallization is at the frontier of chemical engineering, material science, and biochemical research and is affected by many factors. The precise regulation and control of microscale crystal processes is still a major challenge. In the heterogeneous induced nucleation process, the chemical and micro/nanostructural characteristics of the interface play a dominant role. Ideal crystal products can be obtained by modifying the interface characteristics, which has been proven to be a promising strategy. This review illustrates the application of interface properties, including chemical characteristics (hydrophobicity and functional groups) and the morphology of micro/nanostructures (rough structure and cavities, pore shape and pore size, surface porosity, channels), in various microscale crystallization controls and process intensification. Finally, possible future research and development directions are outlined to emphasize the importance of interfacial crystallization control and regulation for crystal engineering.

关键词： interfacial crystallization     heterogeneous nucleation     supersaturation     micro/nanostructure     process control and intensification    

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Calculating frictional force with considering material microstructure and potential on contact surfaces

XU Zhongming, HUANG Ping

《机械工程前沿（英文）》 2007年 第2卷 第4期   页码 474-477 doi: 10.1007/s11465-007-0082-y

摘要： A method based on the energy dissipation mechanism of an Independent Oscillator model is used to calculate the frictional force and the friction coefficient of interfacial friction. The friction work is calculated with considering the potential change of contact surfaces during sliding. The potential change can be gained by a universal adhesive energy function. The relationships between frictional force and parameters of a tribo-system, such as surface energy and microstructure of interfacial material, are set up. The calculation results of the known experimental data denote that the frictional force is nearly proportional to the surface energy of the material, nearly inversely proportional to the scaling length, and independent of the lattice constant. The results agree with that of adhesion friction equations. They also agree with the experimental results performed with an atomic-force microscope under the ultra high vacuum condition.

关键词： coefficient     dissipation mechanism     universal adhesive     interfacial     Independent Oscillator    

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Thin-liquid-film evaporation at contact line

Hao WANG, Zhenai PAN, Zhao CHEN

《能源前沿（英文）》 2009年 第3卷 第2期   页码 141-151 doi: 10.1007/s11708-009-0020-2

摘要： When a liquid wets a solid wall, the extended meniscus near the contact line may be divided into three regions: a nonevaporating region, where the liquid is adsorbed on the wall; a transition region or thin-film region, where effects of long-range molecular forces (disjoining pressure) are felt; and an intrinsic meniscus region, where capillary forces dominate. The thin liquid film, with thickness from nanometers up to micrometers, covering the transition region and part of intrinsic meniscus, is gaining interest due to its high heat transfer rates. In this paper, a review was made of the researches on thin-liquid-film evaporation. The major characteristics of thin film, thin-film modeling based on continuum theory, simulations based on molecular dynamics, and thin-film profile and temperature measurements were summarized.

关键词： meniscus     thin film     contact line     disjoining pressure     evaporation    

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The effects of interfacial strength on fractured microcapsule

Luthfi Muhammad MAULUDIN, Chahmi OUCIF

《结构与土木工程前沿（英文）》 2019年 第13卷 第2期   页码 353-363 doi: 10.1007/s11709-018-0469-3

摘要： The effects of interfacial strength on fractured microcapsule are investigated numerically. The interaction between crack and microcapsule embedded in mortar matrix is modeled based on cohesive approach. The microcapsules are modelled with variation of core-shell thickness ratio and potential cracks are represented by pre-inserted cohesive elements along the element boundaries of the mortar matrix, microcapsules core, microcapsule shell, and at the interfaces between these phases. Special attention is given to the effects of cohesive fracture on the microcapsule interface, namely fracture strength, on the load carrying capacity and fracture probability of the microcapsule. The effect of fracture properties on microcapsule is found to be significant factor on the load carrying capacity and crack propagation characteristics. Regardless of core-shell thickness ratio of microcapsule, the load carrying capacity of self-healing material under tension increases as interfacial strength of microcapsule shell increases. In addition, given the fixed fracture strength of the interface of microcapsule shell, the higher the ratio core-shell thickness, the higher the probability of microcapsules being fractured.

关键词： interfacial strength     cohesive elements     microcapsule     core-shell thickness ratio     fracture properties    

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Modelling of dynamic contact length in rail grinding process

null

《机械工程前沿（英文）》 2014年 第9卷 第3期   页码 242-248 doi: 10.1007/s11465-014-0305-y

摘要：

Rails endure frequent dynamic loads from the passing trains for supporting trains and guiding wheels. The accumulated stress concentrations will cause the plastic deformation of rail towards generating corrugations, contact fatigue cracks and also other defects, resulting in more dangerous status even the derailment risks. So the rail grinding technology has been invented with rotating grinding stones pressed on the rail with defects removal. Such rail grinding works are directed by experiences rather than scientifically guidance, lacking of flexible and scientific operating methods. With grinding control unit holding the grinding stones, the rail grinding process has the characteristics not only the surface grinding but also the running railway vehicles. First of all, it’s important to analyze the contact length between the grinding stone and the rail, because the contact length is a critical parameter to measure the grinding capabilities of stones. Moreover, it’s needed to build up models of railway vehicle unit bonded with the grinding stone to represent the rail grinding car. Therefore the theoretical model for contact length is developed based on the geometrical analysis. And the calculating models are improved considering the grinding car’s dynamic behaviors during the grinding process. Eventually, results are obtained based on the models by taking both the operation parameters and the structure parameters into the calculation, which are suitable for revealing the process of rail grinding by combining the grinding mechanism and the railway vehicle systems.

关键词： rail grinding     contact length     dynamic model     Hamiltonian system     grinding stone     rail grinding car    

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Construction of interfacial dynamic bonds for high performance lignin/polymer biocomposites

《化学科学与工程前沿（英文）》 2023年 第17卷 第10期   页码 1372-1388 doi: 10.1007/s11705-023-2302-3

摘要： Lignin is the largest natural aromatic biopolymer, but usually treated as industrial biomass waste. The development of lignin/polymer biocomposites can promote the high value utilization of lignin and the greening of polymers. However, the weak interfacial interaction between industrial lignin and polymer induces poor compatibility and serious agglomeration in polymer owing to the strong intermolecular force of lignin. As such, it is extremely difficult to prepare high performance lignin/polymer biocomposites. Recently, we proposed the strategy of in situ construction of interfacial dynamic bonds in lignin/polymer composites. By taking advantage of the abundant oxygen-containing polar groups of lignin, we inserted dynamic bonding connection such as hydrogen bonds and coordination bonds into the interphase between lignin and the polymer matrix to improve the interfacial interactions. Meanwhile, the natural amphiphilic structure characteristics of lignin were utilized to construct the hierarchical nanophase separation structure in lignin/polymer composites. The persistent problems of poor dispersity and interfacial compatibility of lignin in the polymer matrix were effectively solved. The lignin-modified polymer composites achieved simultaneously enhanced strength and toughness. This concise review systematically summarized the recent research progress of our group toward building high-performance lignin/polymer biocomposites through the design of interfacial dynamic bonds (hydrogen bonds, coordination bonds, and dynamic covalent bonds) between lignin and different polymer systems (polar plastics, rubber, polyurethane, hydrogels, and other polymers). Finally, the future development direction, main challenges, and potential solutions of lignin application in polymers were presented.

关键词： lignin     polymer     interfacial dynamic bonds    

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Computation and investigation of mode characteristics in nonlinear system with tuned/mistuned contact

Houxin SHE, Chaofeng LI, Qiansheng TANG, Hui MA, Bangchun WEN

《机械工程前沿（英文）》 2020年 第15卷 第1期   页码 133-150 doi: 10.1007/s11465-019-0557-7

摘要： This study derived a novel computation algorithm for a mechanical system with multiple friction contact interfaces that is well-suited to the investigation of nonlinear mode characteristic of a coupling system. The procedure uses the incremental harmonic balance method to obtain the nonlinear parameters of the contact interface. Thereafter, the computed nonlinear parameters are applied to rebuild the matrices of the coupling system, which can be easily solved to calculate the nonlinear mode characteristics by standard iterative solvers. Lastly, the derived method is applied to a cycle symmetry system, which represents a shaft–disk–blade system subjected to dry friction. Moreover, this study analyzed the effects of the tuned and mistuned contact features on the nonlinear mode characteristics. Numerical results prove that the proposed method is particularly suitable for the study of nonlinear characteristics in such nonlinear systems.

关键词： coupling vibration     nonlinear mode     original algorithm     contact interface    

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Transient analysis of thermoelastic contact problem of disk brakes

Ali BELHOCINE, Mostefa BOUCHETARA

《机械工程前沿（英文）》 2013年 第8卷 第2期   页码 150-159 doi: 10.1007/s11465-013-0266-6

摘要：

The main purpose of this study is to analyze the thermomechanical behavior of the dry contact between the brake disk and pads during the braking phase. The simulation strategy is based on computer code ANSYS11. The modeling of transient temperature in the disk is actually used to identify the factor of geometric design of the disk to install the ventilation system in vehicles. The thermal-structural analysis is then used with coupling to determine the deformation established and the Von Mises stresses in the disk, the contact pressure distribution in pads. The results are satisfactory compared to those found in the literature.

关键词： brake disks     heat flux     heat-transfer coefficient     Von Mises stress     contact pressure    

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Experimental study and numerical simulation on compressive buckling behavior of thin steel skins in unilateral contact

Nicholas KEAGE, Christopher MAIOLO, Rebecca PIEROTTI, Xing MA

《结构与土木工程前沿（英文）》 2011年 第5卷 第3期   页码 335-343 doi: 10.1007/s11709-011-0121-y

摘要： In this paper, a practical test and finite element analysis has been undertaken to further investigate the effects of contact buckling. A test rig was designed and constructed to record vertical and transverse deflections of compressively loaded steel skin plates. The boundary conditions were modeled as fully fixed. A finite element analysis was also undertaken using the software package Strand7. Results from both analyses have been examined and compared to data established from previous studies on contact buckling. Both the finite element analysis and practical results correlate well with this data. The result of the investigation has confirmed contact buckling theories and has foreshadowed the onset of the newly observed phenomenon of secondary contact buckling.

关键词： compressive     buckling     thin steel skins     unilateral contact     rigid constraints    

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Computational design of heterogeneous catalysts and gas separation materials for advanced chemical processing

Huaiwei Shi, Teng Zhou

《化学科学与工程前沿（英文）》 2021年 第15卷 第1期   页码 49-59 doi: 10.1007/s11705-020-1959-0

摘要： Functional materials are widely used in chemical industry in order to reduce the process cost while simultaneously increase the product quality. Considering their significant effects, systematic methods for the optimal selection and design of materials are essential. The conventional synthesis-and-test method for materials development is inefficient and costly. Additionally, the performance of the resulting materials is usually limited by the designer’s expertise. During the past few decades, computational methods have been significantly developed and they now become a very important tool for the optimal design of functional materials for various chemical processes. This article selectively focuses on two important process functional materials, namely heterogeneous catalyst and gas separation agent. Theoretical methods and representative works for computational screening and design of these materials are reviewed.

关键词： heterogeneous catalyst     gas separation     solvent     porous adsorbent     material screening and design    

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非连续接触下滚圈的接触压力及疲劳寿命预测

时彧,肖友刚,雷先明

《中国工程科学》 2006年 第8卷 第7期   页码 54-57

摘要：

建立了非连续接触下筒体-滚圈接触压力的计算模型，得出了滚圈弯矩及弯曲应力计算公式。应用名义应力法和局部应力应变法，建立了滚圈疲劳寿命预测模型。通过实例分析，得出了如下结论：通过调窑，将滚圈的最大支承载荷控制在2500kN以内，能显著提高滚圈的疲劳寿命；在传统设计中，将滚圈支承角定为30°不合理；存在一个最佳滚圈支承角，此时滚圈疲劳寿命最大。

关键词： 滚圈     接触压力     支承角     疲劳寿命    

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Application of heterogeneous catalysis to biodiesel synthesis using microalgae oil

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-020-1343-9

摘要：

• Microalgae oil application for biodiesel synthesis is discussed.

关键词： Biodiesel     Heterogeneous catalysis     Transesterification     Microalgae oil    

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Studies on the liquid-liquid interfacial mass transfer process using holographic interferometry

ZHAO Chaofan, ZHU Chunying, MA Youguang

《化学科学与工程前沿（英文）》 2008年 第2卷 第1期   页码 1-4 doi: 10.1007/s11705-008-0006-3

摘要： This paper aims at the interfacial phenomena of liquid-liquid mass transfer and its characteristic. By using the real-time holographic technique, the concentration distributions on the aqueous side were obtained according to holographic diagrams of mass transfer of ethanol through the interface of oil and water at different initial concentrations. Furthermore, the concentrations near the interface and the mass transfer coefficients were attained. A correlation of concentration near the interface to the concentration of the solute in the oil side was proposed. An approach of interfacial energy with solute concentration was established, and the calculated results are at good agreement with the experimental data. It is indicated that the liquid-liquid mass transfer process is approximately in accordance with two-film theory, the interfacial performance may be changed by the addition of the solute, and the interface of liquid-liquid is non-equilibrium thermodynamically during the mass transfer process.

关键词： liquid-liquid     different     real-time holographic     addition     transfer    

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Performance of a hybrid anaerobic-contact oxidation biofilm baffled reactor for the treatment of decentralized

Minmin LIU,Ying ZHAO,Beidou XI,Li’an HOU,Xunfeng XIA

《环境科学与工程前沿（英文）》 2014年 第8卷 第4期   页码 598-606 doi: 10.1007/s11783-013-0576-2

摘要： A novel hybrid anaerobic-contact oxidation biofilm baffled reactor (HAOBR) was developed to simultaneously remove nitrogenous and carbonaceous organic pollutants from decentralized molasses wastewater in the study. The study was based on the inoculation of anaerobic granule sludge in anaerobic compartments and the installation of combination filler in aerobic compartments. The performance of reactor system was studied regarding the hydraulic retention time (HRT), microbial characteristics and the gas water ratio (GWR). When the HRT was 24h and the GWR was 20:1, total ammonia and chemical oxygen demand (COD) of the effluent were reduced by 99% and 91.8%, respectively. The reactor performed stably for treating decentralized molasses wastewater. The good performance of the reactor can be attributed to the high resistance of COD and hydraulic shock loads. In addition, the high solid retention time of contact oxidation biofilm contributed to stable performance of the reactor.

关键词： combination filler     contact oxidation biofilm     food wastewater     anaerobic baffled reactor    

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标题 作者 时间 类型 操作

In-MOF-derived In2S3/Bi2S3 heterojunction for enhanced photocatalytic hydrogen production

期刊论文

Interfacial induction and regulation for microscale crystallization process: a critical review

期刊论文

Calculating frictional force with considering material microstructure and potential on contact surfaces

XU Zhongming, HUANG Ping

期刊论文

Thin-liquid-film evaporation at contact line

Hao WANG, Zhenai PAN, Zhao CHEN

期刊论文

The effects of interfacial strength on fractured microcapsule

Luthfi Muhammad MAULUDIN, Chahmi OUCIF

期刊论文

Modelling of dynamic contact length in rail grinding process

null

期刊论文

Construction of interfacial dynamic bonds for high performance lignin/polymer biocomposites

期刊论文

Computation and investigation of mode characteristics in nonlinear system with tuned/mistuned contact

Houxin SHE, Chaofeng LI, Qiansheng TANG, Hui MA, Bangchun WEN

期刊论文

Transient analysis of thermoelastic contact problem of disk brakes

Ali BELHOCINE, Mostefa BOUCHETARA

期刊论文

Experimental study and numerical simulation on compressive buckling behavior of thin steel skins in unilateral contact

Nicholas KEAGE, Christopher MAIOLO, Rebecca PIEROTTI, Xing MA

期刊论文

Computational design of heterogeneous catalysts and gas separation materials for advanced chemical processing

Huaiwei Shi, Teng Zhou

期刊论文

非连续接触下滚圈的接触压力及疲劳寿命预测

时彧,肖友刚,雷先明

期刊论文

Application of heterogeneous catalysis to biodiesel synthesis using microalgae oil

期刊论文

Studies on the liquid-liquid interfacial mass transfer process using holographic interferometry

ZHAO Chaofan, ZHU Chunying, MA Youguang

期刊论文

Performance of a hybrid anaerobic-contact oxidation biofilm baffled reactor for the treatment of decentralized

Minmin LIU,Ying ZHAO,Beidou XI,Li’an HOU,Xunfeng XIA

期刊论文